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Visible light-driven photocatalytic activity of Cu2O/ZnO/Kaolinite-based composite catalyst for the degradation of organic pollutant

  • Paulos Asefa Fufa
  • , Gebisa Bekele Feysia
  • , Noto Susanto Gultom
  • , Dong Hau Kuo
  • , Xiaoyun Chen
  • , Daniel Manaye Kabtamu
  • , Osman Ahmed Zelekew
  • Adama Science and Technology University
  • National Taiwan University of Science and Technology
  • Fujian Agriculture and Forestry University

Research output: Contribution to journalArticlepeer-review

14 Citations (Scopus)

Abstract

Herein, we design to synthesize a novel Cu2O/ZnO/kaolinite composite catalyst by co-precipitation method. The synthesized composite catalysts were labeled as 5CZK, 10CZK, 15CZK, and 20CZK which represent 5, 10, 15, and 20% of Cu2O, respectively, on ZnO/kaolinite. The photocatalyst samples were characterized with different instruments. Moreover, the methylene blue (MB) dye was used as a target organic pollutant and the degradation was evaluated under visible light irradiation. The highest performance for the degradation of MB was achieved by 10CZK catalyst and degrades 93% within 105 min. However, ZnO (Z), Cu2O/ZnO (CZ), 5CZK, 15CZK, and 20CZK composite catalysts, degrades 28, 66, 76, 71, and 68% of MB dye, respectively. The enhanced degradation efficiency of 10CZK composites catalyst could be due to the higher adsorption properties from metakaolinite and the light-responsive properties of the Cu2O/ZnO samples under visible light. Hence, the resulting composite catalyst could be applicable for environmental remediation.

Original languageEnglish
Article number315601
JournalNanotechnology
Volume33
Issue number31
DOIs
Publication statusPublished - 30 Jul 2022

Keywords

  • CuO
  • Ethiopian clay
  • ZnO
  • kaolinite
  • methylene blue
  • photocatalyst
  • visible light

ASJC Scopus subject areas

  • Bioengineering
  • General Chemistry
  • General Materials Science
  • Mechanics of Materials
  • Mechanical Engineering
  • Electrical and Electronic Engineering

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