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The crystallization kinetics of Er/Yb co-doped oxyfluoride glasses

  • Michal Zelechower
  • , Elwira Czerska
  • , Elzbieta Augustyn
  • , Julian Plewa
  • , Radoslaw Lisiecki
  • , Danuta Stróz
  • , Tomasz Rzychon
  • , Kinga Rodak
  • , Witold Ryba-Romanowski
  • Silesian University of Technology
  • Münster University of Applied Sciences
  • Polish Academy of Sciences
  • University of Silesia in Katowice

Research output: Chapter in Book/Report/Conference proceedingConference contributionpeer-review

3 Citations (Scopus)

Abstract

The intention of the authors is to show a possibility of controlled crystallization of Er/Yb co-doped oxyfluoride glass fibers provided for glass-ceramics core fiber lasers or optical amplifiers at 1550 nm. Selected glasses (the batch composition 48SiO211Al2O3-7Na2CO3-10CaO-10PbO-12PbF2-1.5/0.6YbF3-0.5/0.2ErF3) were examined in the form of powders of diameter 45-100 μm (diameter comparable to that of standard multimode fiber core 62 μm). Powders were annealed at various temperatures and time periods in order to obtain glass-ceramics with different crystalline fraction. DTA measurements and calculations (isothermal and non-isothermal annealing) enabled to determine JMAK (JohnsonMehl-Avrami-Kissinger) equation parameters and to estimate crystal growth rate and certain features of nucleation stage. XRD/TEM/SAED/EDS/HRTEM/SEM/EDS techniques (X-ray diffraction, transmission electron microscopy, scanning electron microscopy, energy dispersive X-ray spectroscopy) enabled to determine crystal structure of growing crystals (erbium and ytterbium enriched hexagonal PbF2, erbium and ytterbium enriched cubic PbF2 isomorphic to the fluorite structure). Luminescence intensity at 1550 nm under 488/980 nm excitation has shown comparable values for glassceramics powder and for bulk glass what suggests a considerably higher emission yield for glass-ceramics fiber. The lifetime of erbium excited state for glass-ceramics powder (∼4 ms) is also comparable to that of bulk glass and is promising from the point of view of a stimulated emission. Computed parameters of JMAK equation enable to establish heat treatment conditions for glass fibers and hence to control the level (fraction) of glass crystallization.

Original languageEnglish
Title of host publicationOptical Fibers and Their Applications 2017
EditorsRyszard S. Romaniuk, Jan Dorosz
PublisherSPIE
ISBN (Electronic)9781510610958
DOIs
Publication statusPublished - 2017
Event17th Optical Fibers and Their Applications 2017, OFTA 2017 - Bialystok, Suprasl, Poland
Duration: 23 Jan 201727 Jan 2017

Publication series

NameProceedings of SPIE - The International Society for Optical Engineering
Volume10325
ISSN (Print)0277-786X
ISSN (Electronic)1996-756X

Conference

Conference17th Optical Fibers and Their Applications 2017, OFTA 2017
Country/TerritoryPoland
CityBialystok, Suprasl
Period23/01/1727/01/17

Keywords

  • Crystal growth
  • Glass-ceramics
  • Nucleation
  • Optical fibers
  • Thermal analysis

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Condensed Matter Physics
  • Computer Science Applications
  • Applied Mathematics
  • Electrical and Electronic Engineering

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