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Effect of the nature of the electrolyte on the properties of unpaired spins in polyaniline

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19 Citations (Scopus)

Abstract

An extended study has been carried out to find the relation between the number of spins, the applied potential and the charge of the doping anion in the case of polyaniline electropolymerized in 5 M tetrafluoroboric acid. It was found that in the presence of acids which supply double-charged anions, a fast recombination of polarons to bipolarons occurs. This is in contrast to single-charged anions which stabilize polarons. Three types of spins were detected in the study: (i) localized spins, formed at the beginning of the oxidation process; (ii) mobile spins existing in the presence of single-charged anions; (iii) spins localized mostly at structural defects.

Original languageEnglish
Pages (from-to)183-194
Number of pages12
JournalSynthetic Metals
Volume35
Issue number1-2
DOIs
Publication statusPublished - 1990

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Condensed Matter Physics
  • Mechanics of Materials
  • Mechanical Engineering
  • Metals and Alloys
  • Materials Chemistry

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